Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Sasaki, Yuji; Kaneko, Masashi; Ban, Yasutoshi; Kinoshita, Ryoma; Matsumiya, Masahiko*; Shinoku, Kota*; Shiroishi, Hidenobu*
Analytical Sciences, 39(9), p.1575 - 1583, 2023/09
Times Cited Count：0 Percentile：0(Chemistry, Analytical)Extraction of Rh from HCl can be performed by NTAamide(C6) (hexahexyl-nitrilotriacetamide) and other related compounds into n-dodecane. We use ion-pair extraction of anionic species of Rh-chloride and protonated extractant. Rh behave as anion in hydrochloric acid and the tertiary nitrogen atom in extractant may be protonated to produce the quaternary amine in acidic condition. From the present work, the maximum distribution ratio of Rh(III) is 16. The D(Rh) values are changeable during preparation of the aqueous solutions because different Rh-Cl-H
O complexes are formed in HCl media and show the slow exchange rate between Cl and HO. Using the UV spectrum, Rh-chloride solution having the peak of spectrum at 504 nm can be extracted effectively, where RhCl
(HO)
and RhCl
(H
O)
exist mainly from DFT calculation. Stoichiometry of one-one complex of Rh and NTAamide is obtained from slope analysis, and 85 mM of concentrated Rh ion can be extracted.
Tamura, Fumihiko; Omori, Chihiro*; Yoshii, Masahito*; Tomizawa, Masahito*; Toyama, Takeshi*; Sugiyama, Yasuyuki*; Hasegawa, Katsushi*; Kobayashi, Aine*; Okita, Hidefumi
Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.175 - 178, 2023/01
J-PARC MR delivers high intensity proton beams to the neutrino experiment. Eight bunches with high peak currents are extracted from the MR by the extraction kicker, therefore the neutrino beam has the similar structure. Intermediate Water Cherenkov Detector (IWCD) will be installed for the future experiments and the IWCD requires a time structure with low peaks. We consider bunch manipulation at flattop of the MR for reducing the peak current. It should be quickly done to avoid the significant loss of the beam power. The beam gap for the kicker rise time must be kept. We propose a non-adiabatic bunch manipulation using the multiharmonic rf voltage. The longitudinal impedance in the MR can affect the beam stability. The feasibility of the manipulation is discussed by using the longitudinal simulations.
Jameson, R. A.*; Yee-Rendon, B.
Journal of Instrumentation (Internet), 17(12), p.P12011_1 - P12011_11, 2022/12
Times Cited Count：0 Percentile：0(Instruments & Instrumentation)A new application of vane modulation variation in a Radio Frequency Quadrupole (RFQ) cell has been applied that significantly improves beam bunching and longitudinal emittance control to achieve lower longitudinal rms emittance at the RFQ output. This procedure occurs in the individual cells, is independent of the overall design, and therefore is general, affording an extra parameter for beam manipulation. It can be applied besides the usual goals of vane modulation variation, e.g., to achieve higher acceleration efficiency. Examples of the cumulative effects on the overall design are provided to point out further exploration avenues for the designer.
Maekawa, Fujio
JAEA-Conf 2022-001, p.7 - 13, 2022/11
The partitioning and transmutation (P-T) technology has promising potential for volume reduction and mitigation of degree of harmfulness of high-level radioactive waste. JAEA is developing the P-T technology combined with accelerator driven systems (ADS). One of critical issues affecting the feasibility of ADS is the proton beam window (PBW) which functions as a boundary between the accelerator and the sub-critical reactor core. The PBW is damaged by a high-intensity proton beam and spallation neutrons produced in the target, and also by flowing high-temperature liquid lead bismuth eutectic alloy which is corrosive to steel materials. To study the materials damage under the ADS environment, J-PARC is proposing a plan of proton irradiation facility which equips with a liquid lead-bismuth spallation target bombarded by a 400 MeV - 250 kW proton beam. The facility is also open for versatile purposes such as soft error testing of semi-conductor devises, RI production, materials irradiation for fission and fusion reactors, and so on. Application to nuclear data research with using the proton beam and spallation neutrons is also one of such versatile purposes, and we welcome unique ideas from the nuclear data community.
Yee-Rendon, B.; Meigo, Shinichiro; Kondo, Yasuhiro; Tamura, Jun; Nakano, Keita; Maekawa, Fujio; Iwamoto, Hiroki; Sugawara, Takanori; Nishihara, Kenji
Journal of Instrumentation (Internet), 17(10), p.P10005_1 - P10005_21, 2022/10
Times Cited Count：0 Percentile：0(Instruments & Instrumentation)To reduce the hazard of minor actinides in nuclear waste, JAEA proposed an accelerator-driven subcritical system (JAEA-ADS). The JAEA-ADS drives a subcritical reactor 800-MWth by 30-MW proton linac delivering the beam to the spallation neutron target inside the reactor. The beam transport to the target (BTT) is required for high-beam power stability and low peak density to ensure the integrity of the beam window. Additionally, the design should have compatible with the reactor design for the maintenance and replacement of the fuel and the beam window. A robust-compact BTT design was developed through massive multiparticle simulations. The beam optics was optimized to guarantee beam window feasibility requirements by providing a low peak density of less than 0.3 
A/mm. Beam stability was evaluated and improved by simultaneously applying the linac's input beam and element errors. The input beam errors to the reactor were based on the beam degradation obtained by implementing fast fault compensation in the linac. Those results show that the BTT fulfills the requirements for JAEA-ADS.
Yamamoto, Kazami; Kinsho, Michikazu; Hayashi, Naoki; Saha, P. K.; Tamura, Fumihiko; Yamamoto, Masanobu; Tani, Norio; Takayanagi, Tomohiro; Kamiya, Junichiro; Shobuda, Yoshihiro; et al.
Journal of Nuclear Science and Technology, 59(9), p.1174 - 1205, 2022/09
Times Cited Count：6 Percentile：84.97(Nuclear Science & Technology)In the Japan Proton Accelerator Research Complex, the purpose of the 3 GeV rapid cycling synchrotron (RCS) is to accelerate a 1 MW, high-intensity proton beam. To achieve beam operation at a repetition rate of 25 Hz at high intensities, the RCS was elaborately designed. After starting the RCS operation, we carefully verified the validity of its design and made certain improvements to establish a reliable operation at higher power as possible. Consequently, we demonstrated beam operation at a high power, namely, 1 MW. We then summarized the design, actual performance, and improvements of the RCS to achieve a 1 MW beam.
Ni and Zr at 0.4, 1.3, 2.2, and 3.0 GeVTakeshita, Hayato*; Meigo, Shinichiro; Matsuda, Hiroki*; Iwamoto, Hiroki; Nakano, Keita; Watanabe, Yukinobu*; Maekawa, Fujio
Nuclear Instruments and Methods in Physics Research B, 527, p.17 - 27, 2022/09
Times Cited Count：2 Percentile：53.91(Instruments & Instrumentation)To improve accuracy of nuclear design of accelerator driven nuclear transmutation systems and so on, nuclide production cross sections on Ni and Zr were measured for GeV energy protons. The measured results were compared with PHITS calculations, JENDL/HE-2007 and so on.
Yee-Rendon, B.; Kondo, Yasuhiro; Tamura, Jun; Nakano, Keita; Maekawa, Fujio; Meigo, Shinichiro
Physical Review Accelerators and Beams (Internet), 25(8), p.080101_1 - 080101_17, 2022/08
Times Cited Count：2 Percentile：52.69(Physics, Nuclear)High reliability and availability are primary goals for the operation of particle accelerators, especially for accelerator-driven subcritical systems (ADS). ADSs employ high-power beams for the transmutation of minor actinide; as a result, the amount and the radiotoxicity of the nuclear waste are considerably reduced. To this end, the Japan Atomic Energy Agency is designing a 30-MW continuous wave (cw) super-conducting proton linear accelerator (linac) that supplies neutrons to an 800-MW subcritical reactor by a spallation process. The major challenge for an ADS linac is the strict control of the beam trip duration and its frequency to avoid thermal stress in the subcritical reactor structures. The maximum allowed beam trips for failures longer than a few seconds are estimated to be far below the rate achieved in current accelerators. Thus, we implemented a combination of hot standby and local compensation that enables a fast beam recovery. This work comprehensively investigated the tolerance of our linac lattice for the local compensations for failures in superconducting cavities and magnets. This scheme includes simultaneous compensation of multiple cavities in independent and same cryomodules that significantly enhance the reliability of the linac. The returned schemes present acceptable beam performance to guarantee the integrity of the linac and the beam transport to the target; moreover, they satisfy the beam stability in the beam window. In addition, the readjusted elements are subjected to moderate stress to ensure a sustainable operation. This manuscript reports the beam dynamics results toward fulfilling the high reliability demanded by an ADS linac.
Yamamoto, Masanobu; Nomura, Masahiro; Okita, Hidefumi; Shimada, Taihei; Tamura, Fumihiko; Hara, Keigo*; Hasegawa, Katsushi*; Omori, Chihiro*; Sugiyama, Yasuyuki*; Yoshii, Masahito*
Proceedings of 13th International Particle Accelerator Conference (IPAC 22) (Internet), p.1336 - 1338, 2022/06
In order to accelerate a high intensity beam in the RCS, a large amplitude of the rf current is provided by a tube amplifier to compensate a heavy beam loading. Tetrode vacuum tubes are used in the RCS, and the control grid voltage enters into a positive region to feed such a large rf current. The positive grid biasing affects the waveform of the control grid voltage; it is deformed due to the induced control grid current under the condition of the multi-harmonic rf driving. Furthermore, the DC bias voltage drop on the control grid is observed because of the exceeding the capability for the control grid power supply. We describe the influence of the positive grid biasing in the RCS.
Maekawa, Fujio; Takei, Hayanori
Purazuma, Kaku Yugo Gakkai-Shi, 98(5), p.206 - 210, 2022/05
In developing an accelerator-driven nuclear transmutation system (ADS), it is necessary to solve technical issues related to proton beams, such as the development of materials that can withstand high-intensity proton beams and the characterization of subcritical cores driven by proton beams. Therefore, at the high-intensity proton accelerator facility J-PARC, a transmutation experimental facility that actually conducts various tests using a high-intensity proton beam is being planned. This paper introduces the outline and future direction of the transmutation experimental facility.
Nakano, Keita; Matsuda, Hiroki*; Meigo, Shinichiro; Iwamoto, Hiroki; Takeshita, Hayato*; Maekawa, Fujio
JAEA-Research 2021-014, 25 Pages, 2022/03
JAEA-Research-2021-014.pdf:2.1MB
For the development of accelerator-driven transmutation system (ADS), measurement of nuclide production cross-sections in proton-induced reactions on 
Be, C, 
Al, 
Sc, and V have been performed. The measured data are compared with the calculations by the latest nuclear reaction models and with the nuclear data library to investigate the reproducibilities.
Lu target irradiated with 0.4-, 1.3-, 2.2-, and 3.0-GeV protonsTakeshita, Hayato; Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Hiroki; Nakano, Keita; Watanabe, Yukinobu*; Maekawa, Fujio
JAEA-Conf 2021-001, p.207 - 212, 2022/03
Prediction of nuclide production of spallation products by high-energy proton injection plays a fundamental and important role in shielding design of high-intensity proton accelerator facilities such as accelerator driven nuclear transmutation system (ADS). Since the prediction accuracy of the nuclear reaction models used in the production quantity prediction simulation is insufficient, it is necessary to improve the nuclear reaction models. We have measured nuclide production cross sections for various target materials with the aim of acquiring experimental data and improving nuclear reaction models. In this study, 1.3-, 2.2- and 3.0-GeV proton beams were irradiated to Lu target, and nuclide production cross-section data were acquired by the activation method. The measured data were compared with several nuclear reaction models used in Monte Carlo particle transport calculation codes to grasp the current prediction accuracy and to study how the nuclear reaction model could be improved.
Yee-Rendon, B.; Kondo, Yasuhiro; Maekawa, Fujio; Meigo, Shinichiro; Tamura, Jun
Physical Review Accelerators and Beams (Internet), 24(12), p.120101_1 - 120101_17, 2021/12
Times Cited Count：3 Percentile：46.8(Physics, Nuclear)The Japan Atomic Energy Agency (JAEA) is working on the research and development of a 30-MW continuous wave (CW) proton linear accelerator (linac) for the JAEA accelerator-driven subcritical system (ADS) proposal. The linac will accelerate a 20 mA proton beam to 1.5 GeV, using mainly superconducting cavities. The main challenge for an ADS accelerator is the high reliability required to prevent thermal stress in the subcritical reactor; thus, we pursue a robust lattice to achieve stable operation. To this end, the beam optics design reduces the emittance growth and the beam halo through the superconducting part of the linac. First, we simulated an ideal machine without any errors to establish the operation conditions of the beam. Second, we applied element errors and input beam errors to estimate the tolerance of the linac design. Finally, we implemented a correction scheme to increase the lattice tolerance by reducing the beam centroid offset on the transverse plane. Massive multiparticle simulations and a cumulative statistic of 1
10
macroparticles have shown that the JAEA-ADS linac can operate with less than 1 W/m beam losses in error scenarios.
Yoshimoto, Masahiro; Nakanoya, Takamitsu; Yamazaki, Yoshio; Saha, P. K.; Kinsho, Michikazu; Yamamoto, Shunya*; Okazaki, Hiroyuki*; Taguchi, Tomitsugu*; Yamada, Naoto*; Yamagata, Ryohei*
Proceedings of 18th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.850 - 854, 2021/10
no abstracts in English
Yee-Rendon, B.; Kondo, Yasuhiro; Maekawa, Fujio; Meigo, Shinichiro; Tamura, Jun
Proceedings of 12th International Particle Accelerator Conference (IPAC 21) (Internet), p.790 - 792, 2021/08
The Medium Energy Beam Transport (MEBT) will transport a CW proton beam with a current of 20 mA and energy of 2.5 MeV from the exit of the normal conducting Radiofrequency Quadrupole (RFQ) to the superconducting Half-Wave resonator (HWR) section. The MEBT must provide a good matching between the RFQ and HWR, effective control of the emittance growth and the halo formation, enough space for all the beam diagnostics devices, among others. This work reports the first lattice design and the beam dynamics studies for the MEBT of the JAEA-ADS.
Yamamoto, Masanobu; Okita, Hidefumi; Nomura, Masahiro; Shimada, Taihei; Tamura, Fumihiko; Furusawa, Masashi*; Hara, Keigo*; Hasegawa, Katsushi*; Omori, Chihiro*; Sugiyama, Yasuyuki*; et al.
Proceedings of 12th International Particle Accelerator Conference (IPAC 21) (Internet), p.1884 - 1886, 2021/08
Tetrode vacuum tubes in J-PARC RCS are used under a reduced filament voltage condition compared with the rating value to prolong the tube lifetime. For the first time after 60,000 hour of operation in the RCS, one tube has reached the end of its life in 2020. Therefore, the reduced filament voltage works well because the tube has been running beyond an expected lifetime suggested by the tube manufacturer. However, the reduced filament voltage decreased the electron emission from the filament. Although the large amplitude of the anode current is necessary for the high intensity beam acceleration to compensate a wake voltage, a solid-state amplifier to drive a control grid circuit almost reaches the output power limit owing to the poor electron emission from the filament. We changed the filament voltage reduction rate from 15% to 5%. The required power of the solid-state amplifier was fairly reduced, whereas the accelerated beam power remained the same. We describe the measurement results of the vacuum tube parameters in terms of the filament voltage tuning.
Takeshita, Hayato; Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Hiroki; Maekawa, Fujio; Watanabe, Yukinobu*
JPS Conference Proceedings (Internet), 33, p.011045_1 - 011045_6, 2021/03
To improve accuracy of nuclear design of accelerator driven nuclear transmutation systems, nuclide production cross sections on Ni and Zr, which were candidate materials to be used in ADS, were measured for GeV energy protons. The measured results were compared with PHITS calculations and JENDL/HE-2007.
for a mercury target induced by 3-GeV protonsMatsuda, Hiroki; Iwamoto, Hiroki; Meigo, Shinichiro; Takeshita, Hayato*; Maekawa, Fujio
Nuclear Instruments and Methods in Physics Research B, 483, p.33 - 40, 2020/11
Times Cited Count：3 Percentile：36.4(Instruments & Instrumentation)A thick target neutron yield for a mercury target at an angle of 180 from the incident beam direction is measured with the time-of-flight method using a 3-GeV proton beam at the Japan Proton Accelerator Research Complex (J-PARC). Comparing the experimental result with a Monte Carlo particle transport simulation by the Particle and Heavy Ion Transport code System (PHITS) shows that there are apparent discrepancies. We find that this trend is consistent with an experimental result of neutron-induced re- action rates obtained using indium and niobium activation foils. Comparing proton-induced neutron-production double-differential cross-sections for a lead target at backward directions between the PHITS calculation and experimental data suggests that the dis- crepancies for our experiments would be linked to the neutron production calculation around 3 GeV by the PHITS spallation model and/or the calculation of nonelastic cross-sections around 3 GeV in the particle transport simulation.
Matsuda, Hiroki; Meigo, Shinichiro; Iwamoto, Yosuke; Yoshida, Makoto*; Hasegawa, Shoichi; Maekawa, Fujio; Iwamoto, Hiroki; Nakamoto, Tatsushi*; Ishida, Taku*; Makimura, Shunsuke*
Journal of Nuclear Science and Technology, 57(10), p.1141 - 1151, 2020/10
Times Cited Count：9 Percentile：75.92(Nuclear Science & Technology)To estimate the structural damages of materials in accelerator facilities, displacement per atom (dpa) is widely employed as a damage index, calculated based on the displacement cross-section obtained using a calculation model. Although dpa is applied as standard, the experimental data of the displacement cross-section for a proton in the energy region above 20 MeV are scarce. Among the calculation models, difference of about factor 8 exist, so that the experimental data of the cross-section are crucial to validate the model. To obtain the displacement cross-section, we conducted experiments at J-PARC. The displacement cross-section of copper and iron was successfully obtained for a proton projectile with the kinetic energies, 0.4 - 3 GeV. The results were compared with those obtained using the widely utilized Norgertt-Robinson-Torrens (NRT) model and the athermal-recombination-corrected (arc) model based on molecular dynamics. It was found that the NRT model overestimates the present displacement cross-section by 3.5 times. The calculation results obtained using with the arc model based on the Nordlund parameter show remarkable agreement with the experimental data. It can be concluded that the arc model must be employed for the dpa calculation for the damage estimation of copper and iron.
Pyeon, C. H.*; Talamo, A.*; Fukushima, Masahiro
Journal of Nuclear Science and Technology, 57(2), p.133 - 135, 2020/02
Times Cited Count：3 Percentile：96.32(Nuclear Science & Technology)